Elastico-mechanoluminescence technology has shown significant application prospects in stress sensing, artificial skin, remote interaction, and other research areas. Its progress mainly lies in realizing stress visualization and two-dimensional or even three-dimensional stress-sensing effects using a passive sensing mode. However, the widespread promotion of mechanoluminescence (ML) technology has been hindered by issues such as high stress or strain thresholds and a single sensing mode based on luminous intensity. In this study, a highly efficient green-emitting ML with dual mode stress-sensing characteristics driven by micro-scale strain was developed using LiTaO 3: Tb 3+. In addition to single-mode sensing based on the luminous intensity, the self-defined parameter (Q) was also introduced as a dual-mode factor for sensing the stress velocity. Impressively, the fabricated LiTaO 3: Tb 3+ film is capable of generating discernible ML signals even when supplied with strains as low as 500 μst. This is the current the minimum strain value that can drive green-emitting ML. Our study offers an ideal photonic platform for exploring the potential applications of rare-earth-doped elastico-ML materials in remote interaction devices, high-precision stress sensors, and single-molecule biological imaging. This article is protected by copyright. All rights reserved.